Acta Physica Polonica B

Vol. 34, No. 22, February 2003, page 1113


Antiferro-Quadrupolar Ordering of 4f-Electron State in the Filled Skutterudite PrFe4P12

L. Hao, K. Iwasa, M. Nakajima, D. Kawana, K. Kuwahara, M. Kohgi, H. Sugawara, T.D. Matsuda, Y. Aoki, H. Sato

Magnetic field induced antiferromagnetic (AF) Bragg reflections and superlattice reflections due to a crystal-structure modulation have been observed simultaneously by neutron diffraction in the low temperature phase of the filled-skutterudite PrFe4P12. The present result demonstrates that 4f electrons of Pr ions undergo antiferro-quadrupolar (AFQ) ordering accompanied by the structural phase transition. The field induced AF magnetic moment has been evaluated as 0.065\mu B at H = 5.0 T.

PACS numbers: 71.27.+a, 61.12.Ld, 75.30.Mb


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